Research output: Contribution to journal › Article › peer-review
Thermal roughening of GaAs surface by unwinding dislocation-induced spiral atomic steps during sublimation. / Kazantsev, D. M.; Akhundov, I. O.; Rudaya, N. S. et al.
In: Applied Surface Science, Vol. 529, 147090, 01.11.2020.Research output: Contribution to journal › Article › peer-review
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TY - JOUR
T1 - Thermal roughening of GaAs surface by unwinding dislocation-induced spiral atomic steps during sublimation
AU - Kazantsev, D. M.
AU - Akhundov, I. O.
AU - Rudaya, N. S.
AU - Kozhukhov, A. S.
AU - Alperovich, V. L.
AU - Latyshev, A. V.
PY - 2020/11/1
Y1 - 2020/11/1
N2 - Surface morphology evolution of flat GaAs epitaxial layers grown on mesa structured substrates is studied under annealing in the presence of a saturated Ga-As melt. At high temperatures T > 700 °C, when the annealing conditions are shifted from the equilibrium towards sublimation, the initially flat surface roughens by unwinding spiral monatomic steps, which are induced by screw dislocations. This process leads to the formation of “inverted pyramid” spiral pits. Along with the spiral pits, the roughening consists in multilayer island formation on terraces, at the surface spots where the sublimation is inhibited. The mechanism of island formation is reproduced in the Monte Carlo simulation. The obtained data allowed us to estimate the relative undersaturation of −0.015 and Ga adatom diffusion length of 15 nm at T = 750 °C. Annealing at higher temperature T = 775 °C resulted in a peculiar “vortex”-like surface morphology, which consists in deep spiral pits covering the major part of the surface area.
AB - Surface morphology evolution of flat GaAs epitaxial layers grown on mesa structured substrates is studied under annealing in the presence of a saturated Ga-As melt. At high temperatures T > 700 °C, when the annealing conditions are shifted from the equilibrium towards sublimation, the initially flat surface roughens by unwinding spiral monatomic steps, which are induced by screw dislocations. This process leads to the formation of “inverted pyramid” spiral pits. Along with the spiral pits, the roughening consists in multilayer island formation on terraces, at the surface spots where the sublimation is inhibited. The mechanism of island formation is reproduced in the Monte Carlo simulation. The obtained data allowed us to estimate the relative undersaturation of −0.015 and Ga adatom diffusion length of 15 nm at T = 750 °C. Annealing at higher temperature T = 775 °C resulted in a peculiar “vortex”-like surface morphology, which consists in deep spiral pits covering the major part of the surface area.
KW - GaAs
KW - Screw dislocations
KW - Spiral atomic steps
KW - Surface diffusion length
KW - Surface roughening
KW - PERMEABILITY
KW - GAAS(001) SURFACE
KW - DROPLETS
KW - DENSITY
KW - EVAPORATION
KW - MOTION
KW - HOMOEPITAXIAL GROWTH
KW - SI(111) SURFACE
KW - EQUILIBRIUM
KW - MONTE-CARLO-SIMULATION
UR - http://www.scopus.com/inward/record.url?scp=85087336265&partnerID=8YFLogxK
U2 - 10.1016/j.apsusc.2020.147090
DO - 10.1016/j.apsusc.2020.147090
M3 - Article
AN - SCOPUS:85087336265
VL - 529
JO - Applied Surface Science
JF - Applied Surface Science
SN - 0169-4332
M1 - 147090
ER -
ID: 24716833