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Ni-MOx-Al2O3 (M = Mg, Cr, Ce) catalysts prepared by Pechini technique for low temperature steam reforming of light hydrocarbons into methane-rich gas. / Uskov, S. I.; Potemkin, D. I.; Snytnikov, P. V. et al.

In: Materials Letters, Vol. 221, 15.06.2018, p. 18-21.

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@article{10c9067e7eae4026a72a1b2b0f309917,
title = "Ni-MOx-Al2O3 (M = Mg, Cr, Ce) catalysts prepared by Pechini technique for low temperature steam reforming of light hydrocarbons into methane-rich gas",
abstract = "30 wt.% NiO – 20 wt.% MOx-Al2O3 (M = Mg, Cr, Ce) catalysts with highly disordered structure were prepared by Pechini technique. Reduced catalysts were tested in low temperature steam reforming of model propane-methane mixture into methane-rich gas. The catalysts were compared with industrial samples and exhibited appropriate activity which increased in the following order: Industrial CH4 reforming catalyst < Ni-CeO2-Al2O3 ≈ Ni-Cr2O3-Al2O3 ≈ Ni-Al2O3 < Ni-MgO-Al2O3 ≈ Industrial CO and CO2 methanation catalyst. Ni-MgO-Al2O3 catalyst with lower Ni content and higher calcination and reduction temperatures showed activity close to that of industrial methanation catalyst. The effect was attributed to Ni-MgO interaction which resulted in higher Ni dispersion.",
keywords = "Associated petroleum gas pre-reforming, Interfaces, Low temperature steam reforming, Nanoparticles, Ni-alumina catalyst, Propane pre-reforming, NI/MGO CATALYSTS, PROPANE",
author = "Uskov, {S. I.} and Potemkin, {D. I.} and Snytnikov, {P. V.} and Belyaev, {V. D.} and Bulavchenko, {O. A.} and Simonov, {P. A.} and Sobyanin, {V. A.}",
note = "Publisher Copyright: {\textcopyright} 2018 Elsevier B.V.",
year = "2018",
month = jun,
day = "15",
doi = "10.1016/j.matlet.2018.03.010",
language = "English",
volume = "221",
pages = "18--21",
journal = "Materials Letters",
issn = "0167-577X",
publisher = "Elsevier",

}

RIS

TY - JOUR

T1 - Ni-MOx-Al2O3 (M = Mg, Cr, Ce) catalysts prepared by Pechini technique for low temperature steam reforming of light hydrocarbons into methane-rich gas

AU - Uskov, S. I.

AU - Potemkin, D. I.

AU - Snytnikov, P. V.

AU - Belyaev, V. D.

AU - Bulavchenko, O. A.

AU - Simonov, P. A.

AU - Sobyanin, V. A.

N1 - Publisher Copyright: © 2018 Elsevier B.V.

PY - 2018/6/15

Y1 - 2018/6/15

N2 - 30 wt.% NiO – 20 wt.% MOx-Al2O3 (M = Mg, Cr, Ce) catalysts with highly disordered structure were prepared by Pechini technique. Reduced catalysts were tested in low temperature steam reforming of model propane-methane mixture into methane-rich gas. The catalysts were compared with industrial samples and exhibited appropriate activity which increased in the following order: Industrial CH4 reforming catalyst < Ni-CeO2-Al2O3 ≈ Ni-Cr2O3-Al2O3 ≈ Ni-Al2O3 < Ni-MgO-Al2O3 ≈ Industrial CO and CO2 methanation catalyst. Ni-MgO-Al2O3 catalyst with lower Ni content and higher calcination and reduction temperatures showed activity close to that of industrial methanation catalyst. The effect was attributed to Ni-MgO interaction which resulted in higher Ni dispersion.

AB - 30 wt.% NiO – 20 wt.% MOx-Al2O3 (M = Mg, Cr, Ce) catalysts with highly disordered structure were prepared by Pechini technique. Reduced catalysts were tested in low temperature steam reforming of model propane-methane mixture into methane-rich gas. The catalysts were compared with industrial samples and exhibited appropriate activity which increased in the following order: Industrial CH4 reforming catalyst < Ni-CeO2-Al2O3 ≈ Ni-Cr2O3-Al2O3 ≈ Ni-Al2O3 < Ni-MgO-Al2O3 ≈ Industrial CO and CO2 methanation catalyst. Ni-MgO-Al2O3 catalyst with lower Ni content and higher calcination and reduction temperatures showed activity close to that of industrial methanation catalyst. The effect was attributed to Ni-MgO interaction which resulted in higher Ni dispersion.

KW - Associated petroleum gas pre-reforming

KW - Interfaces

KW - Low temperature steam reforming

KW - Nanoparticles

KW - Ni-alumina catalyst

KW - Propane pre-reforming

KW - NI/MGO CATALYSTS

KW - PROPANE

UR - http://www.scopus.com/inward/record.url?scp=85043992986&partnerID=8YFLogxK

U2 - 10.1016/j.matlet.2018.03.010

DO - 10.1016/j.matlet.2018.03.010

M3 - Article

AN - SCOPUS:85043992986

VL - 221

SP - 18

EP - 21

JO - Materials Letters

JF - Materials Letters

SN - 0167-577X

ER -

ID: 12027767