Generation of a low-temperature plasma in a nozzle to initiate ion-cluster reactions in jets of mixtures of methane with a buffer gas

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Generation of a low-temperature plasma in a nozzle to initiate ion-cluster reactions in jets of mixtures of methane with a buffer gas. / Художитков, Виталий Эдуардович ; Зарвин, Александр Евгеньевич ; Каляда, Валерий Владимирович.

In: E3S Web of Conferences, Vol. 459, 01007, 04.12.2023.

Research output: Contribution to journal › Conference article › peer-review

BibTeX

@article{cab54b5a4e5f4690b280150655d1ed07,

title = "Generation of a low-temperature plasma in a nozzle to initiate ion-cluster reactions in jets of mixtures of methane with a buffer gas",

abstract = "We have considered the option of generating cluster ions directly at the nozzle by initiating an electric discharge. Here, a low-temperature plasma in the flow is formed as a result of the outflow of a partially ionized gas. Conditions for the formation of clusters in the presence of excited particles are provided downstream. To implement this generation option, a scheme for creating an effective discharge in the diffuser part of a supersonic nozzle was proposed and implemented. The diagnostic system of the LEMPUS-2 gas-dynamic facility was adapted to register processes in a supersonic flow of ionized gas with clusters. Molecular nitrogen, which is weakly condensing under experimental conditions, was used as the primary reference gas. The methods of molecular beam mass spectrometry were used to study gas mixtures consisting of 20% methane in an inert carrier gas. Highly condensable argon and practically noncondensable helium were used as carrier gases. It was found that when using the ionized particle selection system for detection, only methane monomers and dimers are registered in mixtures with argon, whereas in mixtures with helium larger clusters are registered. A version of the explanation of the detected dependencies was presented.",

author = "Художитков, {Виталий Эдуардович} and Зарвин, {Александр Евгеньевич} and Каляда, {Валерий Владимирович}",

note = "The work was performed using the shared equipment center {"}Applied physics{"} of the NSU Physics Department with the financial support Ministry of Science and Higher Education of the Russian Federation (FSUS-2020-0039).; XXXIX Сибирский теплофизический семинар ; Conference date: 28-08-2023 Through 31-08-2023",

year = "2023",

month = dec,

day = "4",

doi = "10.1051/e3sconf/202345901007",

language = "English",

volume = "459",

journal = "E3S Web of Conferences",

issn = "2555-0403",

publisher = "EDP Sciences",

}

RIS

TY - JOUR

T1 - Generation of a low-temperature plasma in a nozzle to initiate ion-cluster reactions in jets of mixtures of methane with a buffer gas

AU - Художитков, Виталий Эдуардович

AU - Зарвин, Александр Евгеньевич

AU - Каляда, Валерий Владимирович

N1 - Conference code: XXXIX

PY - 2023/12/4

Y1 - 2023/12/4

N2 - We have considered the option of generating cluster ions directly at the nozzle by initiating an electric discharge. Here, a low-temperature plasma in the flow is formed as a result of the outflow of a partially ionized gas. Conditions for the formation of clusters in the presence of excited particles are provided downstream. To implement this generation option, a scheme for creating an effective discharge in the diffuser part of a supersonic nozzle was proposed and implemented. The diagnostic system of the LEMPUS-2 gas-dynamic facility was adapted to register processes in a supersonic flow of ionized gas with clusters. Molecular nitrogen, which is weakly condensing under experimental conditions, was used as the primary reference gas. The methods of molecular beam mass spectrometry were used to study gas mixtures consisting of 20% methane in an inert carrier gas. Highly condensable argon and practically noncondensable helium were used as carrier gases. It was found that when using the ionized particle selection system for detection, only methane monomers and dimers are registered in mixtures with argon, whereas in mixtures with helium larger clusters are registered. A version of the explanation of the detected dependencies was presented.

AB - We have considered the option of generating cluster ions directly at the nozzle by initiating an electric discharge. Here, a low-temperature plasma in the flow is formed as a result of the outflow of a partially ionized gas. Conditions for the formation of clusters in the presence of excited particles are provided downstream. To implement this generation option, a scheme for creating an effective discharge in the diffuser part of a supersonic nozzle was proposed and implemented. The diagnostic system of the LEMPUS-2 gas-dynamic facility was adapted to register processes in a supersonic flow of ionized gas with clusters. Molecular nitrogen, which is weakly condensing under experimental conditions, was used as the primary reference gas. The methods of molecular beam mass spectrometry were used to study gas mixtures consisting of 20% methane in an inert carrier gas. Highly condensable argon and practically noncondensable helium were used as carrier gases. It was found that when using the ionized particle selection system for detection, only methane monomers and dimers are registered in mixtures with argon, whereas in mixtures with helium larger clusters are registered. A version of the explanation of the detected dependencies was presented.

UR - https://www.scopus.com/record/display.uri?eid=2-s2.0-85182795560&origin=inward&txGid=2c1a9f6ac4ae8b0cb37f085c252ab5e7

UR - https://www.mendeley.com/catalogue/6a5a6b0c-f6f9-316c-bccb-ff58d48ceb4a/

U2 - 10.1051/e3sconf/202345901007

DO - 10.1051/e3sconf/202345901007

M3 - Conference article

VL - 459

JO - E3S Web of Conferences

JF - E3S Web of Conferences

SN - 2555-0403

M1 - 01007

T2 - XXXIX Сибирский теплофизический семинар

Y2 - 28 August 2023 through 31 August 2023

ER -

ID: 59576797