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Reversible Bulk Oxidation of Ni Foil during Oscillatory Catalytic Oxidation of Propane : A Novel Type of Spatiotemporal Self-Organization. / Kaichev, V. V.; Saraev, A. A.; Gladky, A. Yu и др.

в: Physical Review Letters, Том 119, № 2, 026001, 13.07.2017.

Результаты исследований: Научные публикации в периодических изданиях › статья › Рецензирование

Harvard

Kaichev, VV, Saraev, AA, Gladky, AY, Prosvirin, IP, Blume, R, Teschner, D, Hävecker, M, Knop-Gericke, A, Schlögl, R & Bukhtiyarov, VI 2017, 'Reversible Bulk Oxidation of Ni Foil during Oscillatory Catalytic Oxidation of Propane: A Novel Type of Spatiotemporal Self-Organization', Physical Review Letters, Том. 119, № 2, 026001. https://doi.org/10.1103/PhysRevLett.119.026001

APA

Kaichev, V. V., Saraev, A. A., Gladky, A. Y., Prosvirin, I. P., Blume, R., Teschner, D., Hävecker, M., Knop-Gericke, A., Schlögl, R., & Bukhtiyarov, V. I. (2017). Reversible Bulk Oxidation of Ni Foil during Oscillatory Catalytic Oxidation of Propane: A Novel Type of Spatiotemporal Self-Organization. Physical Review Letters, 119(2), [026001]. https://doi.org/10.1103/PhysRevLett.119.026001

Vancouver

Kaichev VV, Saraev AA, Gladky AY, Prosvirin IP, Blume R, Teschner D и др. Reversible Bulk Oxidation of Ni Foil during Oscillatory Catalytic Oxidation of Propane: A Novel Type of Spatiotemporal Self-Organization. Physical Review Letters. 2017 июль 13;119(2):026001. doi: 10.1103/PhysRevLett.119.026001

Author

Kaichev, V. V. ; Saraev, A. A. ; Gladky, A. Yu и др. / Reversible Bulk Oxidation of Ni Foil during Oscillatory Catalytic Oxidation of Propane : A Novel Type of Spatiotemporal Self-Organization. в: Physical Review Letters. 2017 ; Том 119, № 2.

BibTeX

@article{301140f3f641482e8af01685261177b3,
title = "Reversible Bulk Oxidation of Ni Foil during Oscillatory Catalytic Oxidation of Propane: A Novel Type of Spatiotemporal Self-Organization",
abstract = "A novel type of temporal and spatial self-organization in a heterogeneous catalytic reaction is described for the first time. Using in situ x-ray photoelectron spectroscopy, gas chromatography, and mass spectrometry, we show that, under certain conditions, self-sustained reaction-rate oscillations arise in the oxidation of propane over Ni foil because of reversible bulk oxidation of Ni to NiO, which can be observed even with the naked eye as chemical waves propagating over the catalyst surface.",
keywords = "SUSTAINED OSCILLATIONS, NICKEL, KINETICS, WAVES, SPECTROSCOPY, PROPAGATION",
author = "Kaichev, {V. V.} and Saraev, {A. A.} and Gladky, {A. Yu} and Prosvirin, {I. P.} and R. Blume and D. Teschner and M. H{\"a}vecker and A. Knop-Gericke and R. Schl{\"o}gl and Bukhtiyarov, {V. I.}",
year = "2017",
month = jul,
day = "13",
doi = "10.1103/PhysRevLett.119.026001",
language = "English",
volume = "119",
journal = "Physical Review Letters",
issn = "0031-9007",
publisher = "American Physical Society",
number = "2",

}

RIS

TY - JOUR

T1 - Reversible Bulk Oxidation of Ni Foil during Oscillatory Catalytic Oxidation of Propane

T2 - A Novel Type of Spatiotemporal Self-Organization

AU - Kaichev, V. V.

AU - Saraev, A. A.

AU - Gladky, A. Yu

AU - Prosvirin, I. P.

AU - Blume, R.

AU - Teschner, D.

AU - Hävecker, M.

AU - Knop-Gericke, A.

AU - Schlögl, R.

AU - Bukhtiyarov, V. I.

PY - 2017/7/13

Y1 - 2017/7/13

N2 - A novel type of temporal and spatial self-organization in a heterogeneous catalytic reaction is described for the first time. Using in situ x-ray photoelectron spectroscopy, gas chromatography, and mass spectrometry, we show that, under certain conditions, self-sustained reaction-rate oscillations arise in the oxidation of propane over Ni foil because of reversible bulk oxidation of Ni to NiO, which can be observed even with the naked eye as chemical waves propagating over the catalyst surface.

AB - A novel type of temporal and spatial self-organization in a heterogeneous catalytic reaction is described for the first time. Using in situ x-ray photoelectron spectroscopy, gas chromatography, and mass spectrometry, we show that, under certain conditions, self-sustained reaction-rate oscillations arise in the oxidation of propane over Ni foil because of reversible bulk oxidation of Ni to NiO, which can be observed even with the naked eye as chemical waves propagating over the catalyst surface.

KW - SUSTAINED OSCILLATIONS

KW - NICKEL

KW - KINETICS

KW - WAVES

KW - SPECTROSCOPY

KW - PROPAGATION

UR - http://www.scopus.com/inward/record.url?scp=85025479780&partnerID=8YFLogxK

U2 - 10.1103/PhysRevLett.119.026001

DO - 10.1103/PhysRevLett.119.026001

M3 - Article

C2 - 28753346

AN - SCOPUS:85025479780

VL - 119

JO - Physical Review Letters

JF - Physical Review Letters

SN - 0031-9007

IS - 2

M1 - 026001

ER -

ID: 9979329