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Experimental and numerical investigation of the chemical reaction kinetics in H2/CO syngas flame at a pressure of 1–10 atm. / Knyazkov, D. A.; Bolshova, T. A.; Dmitriev, A. M. и др.

в: Combustion, Explosion and Shock Waves, Том 53, № 4, 01.07.2017, стр. 388-397.

Результаты исследований: Научные публикации в периодических изданиях › статья › Рецензирование

Harvard

Knyazkov, DA, Bolshova, TA, Dmitriev, AM, Shmakov, AG & Korobeinichev, OP 2017, 'Experimental and numerical investigation of the chemical reaction kinetics in H2/CO syngas flame at a pressure of 1–10 atm', Combustion, Explosion and Shock Waves, Том. 53, № 4, стр. 388-397. https://doi.org/10.1134/S0010508217040025

APA

Knyazkov, D. A., Bolshova, T. A., Dmitriev, A. M., Shmakov, A. G., & Korobeinichev, O. P. (2017). Experimental and numerical investigation of the chemical reaction kinetics in H2/CO syngas flame at a pressure of 1–10 atm. Combustion, Explosion and Shock Waves, 53(4), 388-397. https://doi.org/10.1134/S0010508217040025

Vancouver

Knyazkov DA, Bolshova TA, Dmitriev AM, Shmakov AG, Korobeinichev OP. Experimental and numerical investigation of the chemical reaction kinetics in H2/CO syngas flame at a pressure of 1–10 atm. Combustion, Explosion and Shock Waves. 2017 июль 1;53(4):388-397. doi: 10.1134/S0010508217040025

Author

Knyazkov, D. A. ; Bolshova, T. A. ; Dmitriev, A. M. и др. / Experimental and numerical investigation of the chemical reaction kinetics in H2/CO syngas flame at a pressure of 1–10 atm. в: Combustion, Explosion and Shock Waves. 2017 ; Том 53, № 4. стр. 388-397.

BibTeX

@article{7b51ddcfad2a463daa8e598957fe4465,
title = "Experimental and numerical investigation of the chemical reaction kinetics in H2/CO syngas flame at a pressure of 1–10 atm",
abstract = "The structure of a premixed stoichiometric flame of syngas (H2/CO/O2/Ar = 0.0667/0.0667/0.0667/0.8) stabilized on a flat burner at a pressure of 5 atm was studied experimentally and by numerical simulation. The mole fraction profiles of the reactants (H2, CO, and O2) and the major (H2O and CO2) and intermediate (O, OH, HO2, and H2O2) combustion products were measured by molecular beam mass spectrometry. The experimental data were compared with those calculated using three detailed chemical-kinetic mechanisms proposed in the literature for oxidation of a H2/CO mixture. Good agreement was found between the results of the experiment and simulation. Calculations of the structure of the flame of the same composition at a pressure of 1 and 10 atm were performed to establish the effect of the pressure on the chemical reaction kinetics in the syngas flame. The results were explained by kinetic analysis of the mechanisms.",
keywords = "high pressure, molecular beam mass spectrometry, numerical simulation, premixed flame, syngas",
author = "Knyazkov, {D. A.} and Bolshova, {T. A.} and Dmitriev, {A. M.} and Shmakov, {A. G.} and Korobeinichev, {O. P.}",
note = "Publisher Copyright: {\textcopyright} 2017, Pleiades Publishing, Ltd.",
year = "2017",
month = jul,
day = "1",
doi = "10.1134/S0010508217040025",
language = "English",
volume = "53",
pages = "388--397",
journal = "Combustion, Explosion and Shock Waves",
issn = "0010-5082",
publisher = "Springer New York",
number = "4",

}

RIS

TY - JOUR

T1 - Experimental and numerical investigation of the chemical reaction kinetics in H2/CO syngas flame at a pressure of 1–10 atm

AU - Knyazkov, D. A.

AU - Bolshova, T. A.

AU - Dmitriev, A. M.

AU - Shmakov, A. G.

AU - Korobeinichev, O. P.

N1 - Publisher Copyright: © 2017, Pleiades Publishing, Ltd.

PY - 2017/7/1

Y1 - 2017/7/1

N2 - The structure of a premixed stoichiometric flame of syngas (H2/CO/O2/Ar = 0.0667/0.0667/0.0667/0.8) stabilized on a flat burner at a pressure of 5 atm was studied experimentally and by numerical simulation. The mole fraction profiles of the reactants (H2, CO, and O2) and the major (H2O and CO2) and intermediate (O, OH, HO2, and H2O2) combustion products were measured by molecular beam mass spectrometry. The experimental data were compared with those calculated using three detailed chemical-kinetic mechanisms proposed in the literature for oxidation of a H2/CO mixture. Good agreement was found between the results of the experiment and simulation. Calculations of the structure of the flame of the same composition at a pressure of 1 and 10 atm were performed to establish the effect of the pressure on the chemical reaction kinetics in the syngas flame. The results were explained by kinetic analysis of the mechanisms.

AB - The structure of a premixed stoichiometric flame of syngas (H2/CO/O2/Ar = 0.0667/0.0667/0.0667/0.8) stabilized on a flat burner at a pressure of 5 atm was studied experimentally and by numerical simulation. The mole fraction profiles of the reactants (H2, CO, and O2) and the major (H2O and CO2) and intermediate (O, OH, HO2, and H2O2) combustion products were measured by molecular beam mass spectrometry. The experimental data were compared with those calculated using three detailed chemical-kinetic mechanisms proposed in the literature for oxidation of a H2/CO mixture. Good agreement was found between the results of the experiment and simulation. Calculations of the structure of the flame of the same composition at a pressure of 1 and 10 atm were performed to establish the effect of the pressure on the chemical reaction kinetics in the syngas flame. The results were explained by kinetic analysis of the mechanisms.

KW - high pressure

KW - molecular beam mass spectrometry

KW - numerical simulation

KW - premixed flame

KW - syngas

UR - http://www.scopus.com/inward/record.url?scp=85028546602&partnerID=8YFLogxK

U2 - 10.1134/S0010508217040025

DO - 10.1134/S0010508217040025

M3 - Article

AN - SCOPUS:85028546602

VL - 53

SP - 388

EP - 397

JO - Combustion, Explosion and Shock Waves

JF - Combustion, Explosion and Shock Waves

SN - 0010-5082

IS - 4

ER -

ID: 9918429