Roles of band gap and Kane electronic dispersion in the terahertz-frequency nonlinear optical response in HgCdTe. / Soranzio, Davide; Abreu, Elsa; Houver, Sarah et al.
In: Physical Review B, Vol. 110, No. 9, 03.09.2024.Research output: Contribution to journal › Article › peer-review
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TY - JOUR
T1 - Roles of band gap and Kane electronic dispersion in the terahertz-frequency nonlinear optical response in HgCdTe
AU - Soranzio, Davide
AU - Abreu, Elsa
AU - Houver, Sarah
AU - Dössegger, Janine
AU - Savoini, Matteo
AU - Teppe, Frédéric
AU - Krishtopenko, Sergey
AU - Mikhailov, Nikolay N.
AU - Dvoretsky, Sergey A.
AU - Johnson, Steven L.
PY - 2024/9/3
Y1 - 2024/9/3
N2 - Materials with linear electronic dispersion often feature high carrier mobilities and unusually strong nonlinear optical interactions. In this work, we investigate the (THz) nonlinear dynamics of one such material, HgCdTe, with an electronic band dispersion heavily dependent on both temperature and stoichiometry. We show how the band gap, carrier concentration and band shape together determine the nonlinear response of the system. At low temperatures, carrier generation from Zener tunneling dominates the nonlinear response with a reduction in the overall transmission. At room temperature, quasiballistic electronic dynamics drive the largest observed nonlinear optical interactions, leading to a transmission increase. Our results demonstrate the sensitivity of these nonlinear optical properties of narrow-gap materials to small changes in the electronic dispersion and carrier concentration.
AB - Materials with linear electronic dispersion often feature high carrier mobilities and unusually strong nonlinear optical interactions. In this work, we investigate the (THz) nonlinear dynamics of one such material, HgCdTe, with an electronic band dispersion heavily dependent on both temperature and stoichiometry. We show how the band gap, carrier concentration and band shape together determine the nonlinear response of the system. At low temperatures, carrier generation from Zener tunneling dominates the nonlinear response with a reduction in the overall transmission. At room temperature, quasiballistic electronic dynamics drive the largest observed nonlinear optical interactions, leading to a transmission increase. Our results demonstrate the sensitivity of these nonlinear optical properties of narrow-gap materials to small changes in the electronic dispersion and carrier concentration.
UR - https://www.mendeley.com/catalogue/ca9bc3d5-de9e-3ed5-aa50-1249053b231d/
U2 - 10.1103/physrevb.110.094303
DO - 10.1103/physrevb.110.094303
M3 - Article
VL - 110
JO - Physical Review B
JF - Physical Review B
SN - 2469-9950
IS - 9
ER -
ID: 60797802