Nonoxidative Conversion of Methane to Aromatic Hydrocarbons in the Presence of ZSM-5 Zeolites Modified with Molybdenum and Rhenium

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Nonoxidative Conversion of Methane to Aromatic Hydrocarbons in the Presence of ZSM-5 Zeolites Modified with Molybdenum and Rhenium. / Stepanov, A. A.; Zaikovskii, V. I.; Korobitsyna, L. L. et al.

In: Petroleum Chemistry, Vol. 59, No. 1, 01.01.2019, p. 91-98.

Research output: Contribution to journal › Article › peer-review

BibTeX

@article{243469599f0d4b3f82bd09cab73cfd32,

title = "Nonoxidative Conversion of Methane to Aromatic Hydrocarbons in the Presence of ZSM-5 Zeolites Modified with Molybdenum and Rhenium",

abstract = "The nonoxidative conversion of methane to aromatic hydrocarbons in the presence of a high-silica ZSM-5 zeolite modified with molybdenum and rhenium nanopowders has been studied. Data on the acid characteristics of the catalysts have been derived by temperature-programmed desorption of ammonia. The microstructure and composition of the Re/ZSM-5 and Re–Mo/ZSM-5 catalyst systems have been studied by transmission electron microscopy. It has been shown that modification of a Mo-containing zeolite with rhenium leads to an increase in the activity and stability of the catalyst in the methane dehydroaromatization reaction.",

keywords = "aromatic hydrocarbons, methane, molybdenum and rhenium nanopowders, natural gas, zeolite, MO, BENZENE, DEHYDROAROMATIZATION, SITES, CATALYSTS, MO/HZSM-5",

author = "Stepanov, {A. A.} and Zaikovskii, {V. I.} and Korobitsyna, {L. L.} and Vosmerikov, {A. V.}",

year = "2019",

month = jan,

day = "1",

doi = "10.1134/S0965544119010146",

language = "English",

volume = "59",

pages = "91--98",

journal = "Petroleum Chemistry",

issn = "0965-5441",

publisher = "Maik Nauka-Interperiodica Publishing",

number = "1",

}

RIS

TY - JOUR

T1 - Nonoxidative Conversion of Methane to Aromatic Hydrocarbons in the Presence of ZSM-5 Zeolites Modified with Molybdenum and Rhenium

AU - Stepanov, A. A.

AU - Zaikovskii, V. I.

AU - Korobitsyna, L. L.

AU - Vosmerikov, A. V.

PY - 2019/1/1

Y1 - 2019/1/1

N2 - The nonoxidative conversion of methane to aromatic hydrocarbons in the presence of a high-silica ZSM-5 zeolite modified with molybdenum and rhenium nanopowders has been studied. Data on the acid characteristics of the catalysts have been derived by temperature-programmed desorption of ammonia. The microstructure and composition of the Re/ZSM-5 and Re–Mo/ZSM-5 catalyst systems have been studied by transmission electron microscopy. It has been shown that modification of a Mo-containing zeolite with rhenium leads to an increase in the activity and stability of the catalyst in the methane dehydroaromatization reaction.

AB - The nonoxidative conversion of methane to aromatic hydrocarbons in the presence of a high-silica ZSM-5 zeolite modified with molybdenum and rhenium nanopowders has been studied. Data on the acid characteristics of the catalysts have been derived by temperature-programmed desorption of ammonia. The microstructure and composition of the Re/ZSM-5 and Re–Mo/ZSM-5 catalyst systems have been studied by transmission electron microscopy. It has been shown that modification of a Mo-containing zeolite with rhenium leads to an increase in the activity and stability of the catalyst in the methane dehydroaromatization reaction.

KW - aromatic hydrocarbons

KW - methane

KW - molybdenum and rhenium nanopowders

KW - natural gas

KW - zeolite

KW - MO

KW - BENZENE

KW - DEHYDROAROMATIZATION

KW - SITES

KW - CATALYSTS

KW - MO/HZSM-5

UR - http://www.scopus.com/inward/record.url?scp=85064543947&partnerID=8YFLogxK

U2 - 10.1134/S0965544119010146

DO - 10.1134/S0965544119010146

M3 - Article

AN - SCOPUS:85064543947

VL - 59

SP - 91

EP - 98

JO - Petroleum Chemistry

JF - Petroleum Chemistry

SN - 0965-5441

IS - 1

ER -

ID: 19630449